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Figure 8.4. Patterned photoalignment of mesochannels using a photomask. Photomask (top) and the obtained silica lm (bottom). Reprinted with permission from the American Chemical Society.

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columns via the p p stacking, rather than rodlike micelles via the hydrophobic effect. The resultant columnar structure of the dye aggregate forms lyotropic mesophases. Recently, such chromonic mesophases have been attracting great attention because of their potential utilities for fabrication of optical elements. The photoalignment of azo dye aggregate by the command surface was rst demonstrated by Ichimura et al. (1995). Further investigations reveal that the photoaligning of the resulting dry lm is achieved in the lyotropic state (Fujiwara and Ichimura, 2002; Ichimura et al., 2002). The dried lms, via chromonic LC of an anionic bis-azo dye, C.I. Direct Blue 67 (B67), have been found to be aligned and patterned by the alignment layer that is preirradiated with LPL (Ruslim et al., 2004; Matsunaga et al., 2003, 2002). The fundamental phase diagrams and mesomorphic properties of B67 have been reported by Ruslim et al. (2003). These innovative ndings are reviewed by Lydon (2004).

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The resulting current is thus positive and proportional to the rate of the metabolic reaction Several types of active transport (also called a pump) can be distinguished Uniport is a type of transport in which only one substance is transported across the membrane An example is the transport of protons across the purple membrane of the halophilic bacterium Halobacterium halobium, where the energy for transport is provided by light activating the transport protein bacteriorhodopsin The calcium pump in the membrane of the rod-shaped cells of the retina is also light-activated; the active substance is the related rhodopsin On radiation, its prosthetic group, retinal, is transformed from the cis form to the trans form and the protein component is protonated by protons from the cytoplasm After several milliseconds, retinal is converted back to the cis form and the protons are released into the surrounding medium.

Nanohybridization of B67 with silica network was recently attempted by Hara et al. (2007). The chromonic LC of B67 was mixed with silica precursor of tetraethoxysilane (TEOS) together with an anionic surfactant (EmalC20) and 2-(2-aminoethoxyl)ethanol (AEE). Here AEE plays an important role in stabilizing the columnar structure of B67. This molecule works as the mediator of the interface between the anionic B67 aggregate and silica. Without AEE, the columnar structure is transformed to a lamella structure in the process of drying (Hara et al., 2007). The optical anisotropy of the nanohybrid lms obviously obeys the direction of the preirradiated LPL to the photocrosslinkable polymer liquid crystal (PPLC) lm, and the effect of ow orientation because the lifting from the sol solution is

Another example of uniport is the functioning of H+-ATPase, described in detail in Section 652 Symport is the interrelated transport of two substances in the same direction, with opposite electrochemical potential gradients Here the energy of the electrochemical potential gradient of one substance is used for active transport of the other substance An example is the combined transport of sodium ions (in the direction of decreasing electrochemical potential) and glucose or amino acid (along its concentration gradient) across the membranes of the cell of the intestinal epithelium In this process, the organism transfers the products of digestion from the intestine into the bloodstream Antiport is the coupling of two opposite transport processes Na + ,K + ATPase activated by magnesium ions is a typical transport protein, enabling transport of sodium and potassium ions against their electrochemical potential gradients.

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This process employs the energy gained from the rupture of the 'macroergic' polyphosphate bond of adenosinetriphosphate (ATP) during its conversion to adenosinediphosphate (ADP) which is catalysed by the enzyme, ATPase In the actual process, the asparagine unit of the enzyme is first phosphorylated with simultaneous conformational changes, connected with the transfer of sodium ions from the cell into the intercellular fluid The second step involves dephosphorylation of the.

Figure 8.5. Photoalignment of chromonic LC/silica nanohybrid. Chemical structure of the component and a scheme of B67 columns on a photoaligned PPLC lm. See color insert.

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