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chiral azobenzene compounds were synthesized by introducing different chiral groups into the same azobenzene group via ester bond without any spacers (Fig. 10.7). HTPs of some chiral compounds without azobenzene group are given in Table 10.2. It is noteworthy that HTP is increased by the introduction of the azobenzene group into the chiral compounds. This may be due to the enhancement of the intermolecular interaction between chiral molecule and LC molecule by the introduction of the azobenzene group with the rod shape. The molecular long axis and molecular aspect ratio are increased by the introduction of the azobenzene group. The molecular length (L) and diameter (D) estimated from the models obtained by MOPAC/PM3 method are given in Table 10.1. The molecular aspect ratio (L/D), which is de ned as the ratio of the molecular length to the molecular diameter of chiral azobenzene molecules, is a measure of anisotropy of the molecular shapes. The anisotropy in the molecular shape is one of the important parameters for appearance of LC phases (Onsager, 1949). In other words, the molecular aspect ratio is related to the anisotropic intermolecular interaction between the chiral and the LC molecules. Therefore, the higher the molecular aspect ratio becomes, the higher HTP of the chiral compounds becomes. Figure 10.9 shows the snapshot after 100 ps of mixture of 5CB/p-azo-9 (98/ 2 mol%) obtained by MD simulation. It seems likely that p p stacking interaction between 5CB molecules is enhanced through the intermolecular interaction between the chiral azobenzene molecule and 5CB molecule. As a result, the order parameter, S, was increased by mixing trans-p-azo-9 in 5CB. However, S of 5CB mixed with cis-p-azo-9 was almost constant. The molecular orientation of the LC molecules doped with the trans-azobenzene is stable relatively to that doped with

If the system considered is closed and thermally insulated, then its entropy increases during a transport phenomenon

The area inside a blade chassis is tight, so space is always a consideration. Most vendors allow up to two small form factor (SFF) 2.5-inch disk drives on their blades. A number of disk drive options are available in this form factor. The most frequently used onboard drives include SFF serial-attached SCSI

TA B L E 1 0 . 1 . HTPs [( 108 m 1 mol 1 g-E44), Experimental], the Length of the Long Axis, L, and the Diameter, D [(A), Measured from Molecular Orbital Calculation with PM3 Method], Data of Chiral Azobenzene Compounds

(2.3.1)

If the system is neither closed nor thermally insulated, then the change in the entropy with time consists of two quantities: of the time change in the entropy as a result of processes occurring within the system St and of entropy changes in the surroundings, caused by transfer of the entropy from the system in the reversible process S"e

* * *

7

dt dt dt If we consider a system of infinitesimal dimensions, then the entropy balance can be described directly by Eq. (2.2.13):

Azo chiral:

(SAS) drives and SFF Serial ATA (SATA) drives, which are both hot-pluggable. The hot-pluggable feature is important because the disk drive is the only moving part on the blade and is more prone to failure. To minimize downtime due to disk failure, blade companies have started providing RAID (redundant arrays of independent disk) controllers that will stripe (for performance) and mirror (for redundancy) the data across the two disks. Many vendors also offer blade storage expansion units, which take up another blade slot that support a number of 3.5-inch HDDs as well as adapters for additional I/O daughter cards.

(2.3.2) }

the cis-azobenzene. Thus, the shape of the azobenzene molecule in uences the molecular orientation of a host LC (Sanpei, 2005).

p^=-divJ5 + a (2.3.3) at where s is the entropy of the system, related to 1 kg of substance, Js is the entropy flux and o is the rate of entropy production per unit volume. The first term on the right-hand side of this equation corresponds to dSJdt and the second to dSJdt in Eq. (2.3.2). The rate of entropy formation for a single transport process (Eq. 2.1.1) is given as

External storage comes in a variety of configurations with a number of different protocols used for access. The two primary methods used are network attached storage (NAS) and storage area Nntworks (SAN).

In binary Ch LC systems consisting of the chiral compound and the host nematic LC, the intermolecular interaction between the chiral azobenzene molecule and LC molecule contributes to HTP of the chiral azobenzene compounds. In this section, photoswitching behavior of some chiral azobenzene compounds (Fig. 10.7) is examined in terms of the in uence of the chiral groups on the photochemical change in HTP. Figure 10.10 shows changes in absorption spectra of p-azo-7 in methanol and in E44 by UV irradiation. The absorption spectra are characterized by a strong absorption at 370 nm corresponding to p p* transition of trans form and a weak absorption at 450 nm, which originates from the n p* transition of cis form. Upon UV irradiation, absorbance at B370 nm was decreased because of the trans cis photoisomerization with an increase in low intensity band at around 450 nm.

o = ~3X = ^LX2 (2.3.4)

Change in the orientation order S by replacing with different chiral dopant. Host/Dopant 5CB 5CB /trans-p-Azo-9 5CB /cis-p-Azo-9 Ratio, mol/mol 50/0 49/1 49/1 S Before 0.53 0.53 0.53 After 0.51 0.66 0.54 S, % 3.8 +19.7 +1.9

(unit J m ' V 1 ^ 1 ) . X is the absolute value of the vector of the driving force X. Generally,

Network Attached Storage (NAS)

o = ^ 2 J,X; = ^ 2 2 UXiX*

Figure 10.9. Snapshots before [(a) trans, (c) cis] and after 100 ps [(b) trans, (d) cis] of mixed LCs (5CB/p-azo-9 = 49/1).