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limited at the molecular level but ampli ed to regulate the MPS structure of the larger feature size. Understanding the interplay between different size hierarchies with retention of dynamic features should be a signi cant issue to create future soft materials. The nanopatterned surface of block copolymer lms can be applied as a template surface to fabricate various functional materials, including biological macromolecules (Kumar and Harn, 2005), conjugated polymers (Goren and Lennox, 2001), inorganic materials (Kim et al., 2004; Spatz et al., 1998), and metals (Fahmi and Stamm, 2005). When such patterns are tuned by light, more complicated and hierarchical structures that will be more suited for device fabrication would be realized. The topics dealt with in this chapter are mostly limited to 2-D systems, but the ultimate goal would be to create sophisticated dynamic 3-D systems similar to the biological ones. It is anticipated that studies on the motions of photoresponsive lms in the assembled states can give proper clues to such future directions.

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the point of view of acid-base properties, solvents can be classified as protic containing a dissociable proton and aprotic not able to dissociate a proton. This classification roughly corresponds to division on the basis of whether the solvent molecules are or are not bonded by hydrogen bonds in the liquid state. Most protic solvents have both protogenic and protophilic character, i.e. they can split off as well as bind protons. They are called, therefore, amphiprotic. These include: water, alcohols, acids (especially carboxylic), ammonia, dimethylsulphoxide and acetonitrile. Solvents that are protogenic and have weak or practically negligible protophilic character include acid solvents, such as sulphuric acid, hydrogen fluoride, hydrogen cyanide, and formic acid. Aprotic solvents are not protogenic, but can be protophilic, e.g. acetone, 1,4-dioxan, tetrahydrof uran, dimethy Iformamide, hexamethylphosphortriamide, propylene carbonate and sulpholane. Solvents that do not participate in protolytic reactions, i.e. do not donate or accept a proton, are usually chemically inert, such as benzene, chlorobenzene, chloroform, tetrachloromethane, etc. The molecules of amphiprotic solvents which are the most important will be designated as SH. Self-ionization occurs to a small degree in these solvents according to the equation 2HS^H 2 S + + S" (1.4.2)

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Advincula RC, Brittain WJ, Caster KC, Ruhe J, editors. 2004. Polymer Brushes. Weinheim: Wiley VCH. Edmondoson S, Osborne VL, Huck WTS. 2004. Polymer brushes via surface initiated polymerizations. Chem Soc Rev 33:14 22. Fahmi AW, Stamm M. 2005. Spatially correlated metallic nanostructures on self assembled diblock copolymer templates. Langmuir 21:1062 1066. Fujiwara T, Ichimura K. 2002. Surface assisted photoalignment control of lyotropic liquid crystals. Part 2. Photopattterning of aqueous solutions of a water soluble anti asthmatic drug as lyotropic liquid crystals. J Mater Chem 12:3387 3391. Fukuda K, Seki T, Ichimura K. 2002a. Photoorientation of poly(di n hexylsilane) by azobenzene monolayer 1. Preparative conditions of poly(di n hexylsilane) spincast lms. Macromolecules 35:2177 2183. Fukuda K, Seki T, Ichimura K. 2002b. Photoorientation of poly(di n hexylsilane) by azobenzene monolayer 2. Structural optimization of the surface azobenzene monolayer. Macromolecules 35:1951 1957. Fukuda T, Matsuda H, Shiraga T, Kimura T, Kato M, Viswanathan N, Kumar J, Tripathy SK. 2000. Photofabrication of surface relief grating on lms of azobenzene polymer with different dye functionalization. Macromolecules 33:4220 4225. Fukumoto H, Nagano S, Kawatsuki N, Seki T. 2005. Photo orientation of mesoporous silica thin lms on photo crosslinkable polymer lm. Adv Mater 17:1035 1039. Fukumoto H, Nagano S, Kawatsuki N, Seki T. 2006. Photoalignment behavior of mesoporous silica thin lms synthesized on a photo crosslinkable polymer lm. Chem Mater 18:1226 1234. Geue T, Zieglar A, Stumpe J. 1997. Light induced orientation phenomena in Langmuir Blodgett multilayers. Macromolecules 30:5729 5738. Goren M, Lennox RB. 2001. Nano scale polypyrol patterns using block copolymer micelles as templates. Nano Lett 1:735 738.

This equilibrium is characterized by the ion product of the solvent thermodynamic ( or apparent ) ( ) (1.4.3)

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