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subsequent rinsing with tetrahydrofuran (THF) (after extraction). As shown, the absorption maximum of the p p* band in the trans form of Az positioned at 356 nm fully disappears after the extraction. Thus, 8Az-4Im molecules are completely eliminated from the lm. AFM scans reveal that the periodic structure is exactly maintained on the lm. The selective extraction of the 8Az-4Im molecules gives rise to a drastic reduction in the peak-to-valley height difference of SRG from 250 to 50 nm because of the volume contraction. The degree of volume contraction almost agrees with the loss of the 8Az-4Im mass. The present proposal can be a facile and versatile method for bleaching the SRG lm.

The explanation of the effect of uncouplers strongly supports the Mitchell theory of oxidative phosphorylation The difference in the hydrogen ion electrochemical potential, formed in bacteria similarly as in mitochondria, can be used not only for synthesis of ATP but also for the electrogenic (connected with net charge transfer) symport of sugars and amino acids, for the electroneutral symport of some anions and for the sodium ion/hydrogen ion antiport, which, for example, maintains a low Na+ activity in the cells of the bacterium Escherichia coli It should be noted that, while the Mitchell theory explains some of the basic characteristics of oxidative phosphorylation, a number of phenomena connected with this process remain unclear from both the biochemical and the electrochemical points of view Biochemical processes in the mitochondrial membrane are still far from being clarified completely.

Microphase separation (MPS) leading to regular patterns at nanometer levels formed by block copolymers in thin lms has recently been a subject of intensive study. Such nanostructures allow for fabrication of even smaller feature sizes than those obtained by the conventional photolithography process, and have potentials for future nanofabrications (Lazzari et al., 2006). Attempts to create active and photocontrollable MPS systems are a fascinating challenge.

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Although the Mitchell theory is called electrochemical, it is obvious that it was not formulated by an electrochemist It employs only thermodynamic quantities and does not consider the kinetics of the individual steps Charge balance is neglected in charge transfer across the mitochondrial membrane, although it is obvious that part of the transferred charge must be consumed in charging the electrical double layer at the membrane surface, which is very diversified; because of the presence of cristae the capacity of the double layer is large The role of transferred protons in acid-base equilibria is also not clear Nonetheless, the Mitchell theory has been a great step forward The second basic bioenergetic process consists of consumption of solar radiation as a source of energy in the organisms.

Earlier investigations revealed that PVAs possessing an Az-containing side chain show large photoinduced area changes on a water surface (Seki et al., 1998, 1996). In a particular case, the monolayer exhibits ca. threefold expansion and contraction by alternating illumination with UV and visible light in a fully reversible manner. This effect can be explained by the polarity change of the Az unit. The molecular packing model exactly explains the degree of area changes, indicating that the macrosize effect correctly re ects the molecular events. In situ X-ray re ectivity (XR) analysis on the water surface by Kago et al. (1999) revealed the actual thickness change on water. Quite recently, Ohe et al. (2007) directly evaluated the photomodulated orientations of the individual chemical bonds of this polymer in detail by sum frequency generation spectroscopy. It is anticipated that, when one of the blocks is composed of a photoresponsive segment (area-variable component) in the monolayer state, the change in the area fraction of the blocks may alter the MPS nanostructures. By utilizing the photomechanical response of the monolayer mentioned earlier, such light-induced modulations in the 2-D nanostructures have been actually attained (Kadota et al., 2005) (Fig. 8.16). The trans and cis isomeric states of Az result in dot and strip structures, respectively, of the Az-containing domain in a reversible manner. This tunable behavior of the morphology provides an important aspect on the chain conformation on water. The middle block of poly(ethylene oxide) (PEO) chain should adopt predominantly loop conformations rather than bridge ones. This fact coincides with the tendency of segregation rather than interpenetration of polymer chains in the 2-D state (Sato et al., 1998). At highly humidi ed state, the morphological changes on a hydrophilic solid surface of mica are also observed

One of the ways of employing solar radiation energy in the organism has already been mentioned in connection with the explanation of the function of the purple membrane of Halobacterium halobium (page 450); however, a far more important means of employing this energy for bioenergetic purposes is photosynthesis.